Contrail formation for aircraft with hydrogen combustion - Part 1: A systematic microphysical investigation

Abstract

The number of ice crystals formed during the contrail's jet phase has a long-lasting impact on the life cycle and radiative forcing of contrail cirrus clouds. For conventional kerosene combustion, suitable parameterizations for early ice crystal number have been developed and employed in general circulation models that are used to estimate the climate impact of contrail cirrus. However, a parameterization for the number of ice crystals formed is lacking for hydrogen combustion. To develop such a parameterization, we present a comprehensive set of contrail formation simulations using the particle-based Lagrangian Cloud Module in a box model approach. Unlike kerosene combustion, no soot particles are emitted. Thus, ice crystals are assumed to form on ambient aerosols entrained into the exhaust plume. The total number of entrained particles primarily governs the nonlinear depletion of water vapor. Consequently, the impact of coarse-mode particles is negligible due to their low abundance. Additionally, ice crystal formation from multiple aerosol populations can be reconstructed from single-population simulations using population-specific properties (size and hygroscopicity) and the total number concentration. We also identify atmospheric conditions where homogeneous droplet nucleation can be safely neglected as potential ice formation pathway. Based on more than 20 000 simulations covering a broad range of atmospheric conditions and aerosol properties, we identify a regime where ice crystal formation becomes nearly independent of ambient relative humidity, aerosol size, and hygroscopicity. Our results provide a basis for a data-driven parameterization of ice crystal number in contrails from hydrogen combustion, to be presented in a companion paper.