Negative dynamic conductivity of the photoinduced eta pairing state

Abstract

We report the observation of a sharp dynamic negative optical conductivity, $\sigma(\omega; t)$, above the equilibrium Mott gap $\omega > \Delta_{\rm c}$, after an electromagnetic pump pulse in the half-filled Hubbard chain. The negative peak in the real part of $\sigma(\omega; t)$ is a distinctive hallmark of the photoinduced $\eta$-pairing state, distinguishing it from phases dominated by incoherent doublon formation, which do not exhibit this feature. The negative conductivity and its dynamic oscillations, observed in the absence of continuous driving, are indicative of a nonequilibrium excitation, akin to the Higgs mode observed in s- and d-wave superconductors. We use the time-dependent tensor-network algorithm in the infinite matrix-product-state representation, providing a detailed characterization of the optical response in this nonequilibrium state.