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Evaluation of the coupled high-resolution atmospheric chemistry model system MECO(n) using in situ and MAX-DOAS NO2 measurements

Kumar, Vinod and Remmers, Julia and Beirle, Steffen and Fallmann, Joachim and Kerkweg, Astrid and Lelieveld, Jos and Mertens, Mariano and Pozzer, Andrea and Steil, Benedikt and Barra, Marc and Tost, Holger and Wagner, Thomas (2021) Evaluation of the coupled high-resolution atmospheric chemistry model system MECO(n) using in situ and MAX-DOAS NO2 measurements. Atmospheric Measurement Techniques (AMT), 14 (7), pp. 5241-5269. Copernicus Publications. doi: 10.5194/amt-14-5241-2021. ISSN 1867-1381.

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Official URL: https://amt.copernicus.org/articles/14/5241/2021/

Abstract

We present high spatial resolution (up to 2.2×2.2 km2) simulations focussed over south-west Germany using the online coupled regional atmospheric chemistry model system MECO(n) (MESSy-fied ECHAM and COSMO models nested n times). Numerical simulation of nitrogen dioxide (NO2) surface volume mixing ratios (VMRs) are compared to in situ measurements from a network with 193 locations including background, traffic-adjacent and industrial stations to investigate the model's performance in simulating the spatial and temporal variability of short-lived chemical species. We show that the use of a high-resolution and up-to-date emission inventory is crucial for reproducing the spatial variability and resulted in good agreement with the measured VMRs at the background and industrial locations with an overall bias of less than 10 %. We introduce a computationally efficient approach that simulates diurnal and daily variability in monthly-resolved anthropogenic emissions to resolve the temporal variability of NO2.

Item URL in elib:https://elib.dlr.de/143404/
Document Type:Article
Title:Evaluation of the coupled high-resolution atmospheric chemistry model system MECO(n) using in situ and MAX-DOAS NO2 measurements
Authors:
AuthorsInstitution or Email of AuthorsAuthor's ORCID iD
Kumar, VinodMax Planck Institute for Chemistry, Mainz, GermanyUNSPECIFIED
Remmers, JuliaMPI MainzUNSPECIFIED
Beirle, Steffensteffen.beirle (at) mpic.deUNSPECIFIED
Fallmann, Joachim2Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, GermanyUNSPECIFIED
Kerkweg, AstridFZ Jülichhttps://orcid.org/0000-0002-8378-3498
Lelieveld, JosMax Planck Institut für Chemie, Mainzhttps://orcid.org/0000-0001-6307-3846
Mertens, MarianoDLR, IPAhttps://orcid.org/0000-0003-3549-6889
Pozzer, AndreaAtmospheric Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germanyhttps://orcid.org/0000-0003-2440-6104
Steil, BenediktBenedikt.Steil (at) mpic.deUNSPECIFIED
Barra, MarcInstitute of Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, GermanyUNSPECIFIED
Tost, HolgerUniv. Mainzhttps://orcid.org/0000-0002-3105-4306
Wagner, Thomasthomas.wagner (at) mpic.deUNSPECIFIED
Date:July 2021
Journal or Publication Title:Atmospheric Measurement Techniques (AMT)
Refereed publication:Yes
Open Access:Yes
Gold Open Access:Yes
In SCOPUS:Yes
In ISI Web of Science:Yes
Volume:14
DOI:10.5194/amt-14-5241-2021
Page Range:pp. 5241-5269
Publisher:Copernicus Publications
ISSN:1867-1381
Status:Published
Keywords:Emissionen Luftqualität NO2
HGF - Research field:Aeronautics, Space and Transport
HGF - Program:Transport
HGF - Program Themes:Transport System
DLR - Research area:Transport
DLR - Program:V VS - Verkehrssystem
DLR - Research theme (Project):V - Transport und Klima
Location: Oberpfaffenhofen
Institutes and Institutions:Institute of Atmospheric Physics > Earth System Modelling
Deposited By: Mertens, Mariano
Deposited On:03 Aug 2021 09:45
Last Modified:03 Aug 2021 09:45

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