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Nitric acid trihydrate nucleation and denitrification in the Arctic stratosphere

Grooss, Jens-Uwe and Engel, Ines and Borrmann, Stefan and Frey, W. and Günther, G. and Hoyle, Christopher and Kivi, Rigel and Luo, B.P. and Molleker, S. and Peter, Thomas and Pitts, C.M. and Schlager, Hans and Stiller, Gabriele and Vömel, H. and Walker, K.A. and Müller, Rolf (2014) Nitric acid trihydrate nucleation and denitrification in the Arctic stratosphere. Atmospheric Chemistry and Physics (14), pp. 1055-1073. Copernicus Publications. DOI: 10.5194/acp-14-1055-2014 ISSN 1680-7316

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Official URL: http://www.atmos-chem-phys.net/14/1055/2014/acp-14-1055-2014.html

Abstract

Nitric acid trihydrate (NAT) particles in the polar stratosphere have been shown to be responsible for vertical redistribution of reactive nitrogen (NOy). Recent observations by Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) aboard the CALIPSO satellite have been explained in terms of heterogeneous nucleation of NAT on foreign nuclei, revealing this to be an important formation pathway for the NAT particles. In state of the art global- or regional-scale models, heterogeneous NAT nucleation is currently simulated in a very coarse manner using a constant, saturation-independent nucleation rate.

Item URL in elib:https://elib.dlr.de/93244/
Document Type:Article
Title:Nitric acid trihydrate nucleation and denitrification in the Arctic stratosphere
Authors:
AuthorsInstitution or Email of AuthorsAuthors ORCID iD
Grooss, Jens-UweForschungszentrum JülichUNSPECIFIED
Engel, InesForschungszentrum JülichUNSPECIFIED
Borrmann, StefanMPI für Chemie, MainzUNSPECIFIED
Frey, W.MPI für Chemie, MainzUNSPECIFIED
Günther, G.FZ Jülich, JülichUNSPECIFIED
Hoyle, ChristopherETH Zürich, Zürich, CHUNSPECIFIED
Kivi, RigelFinnish Meteorological Institute, Sodankylä, FIUNSPECIFIED
Luo, B.P.ETH Zürich, Zürich, CHUNSPECIFIED
Molleker, S.Uni MainzUNSPECIFIED
Peter, ThomasETH, Zürich, CHUNSPECIFIED
Pitts, C.M.NASA Langley Research Center, Hampton, VA, USAUNSPECIFIED
Schlager, HansDLR, IPAUNSPECIFIED
Stiller, GabrieleIMK KarlsruheUNSPECIFIED
Vömel, H.DWD, LindenbergUNSPECIFIED
Walker, K.A.Uni Toronto, Toronto, Ontario, CANUNSPECIFIED
Müller, RolfForschungszentrum JülichUNSPECIFIED
Date:2014
Journal or Publication Title:Atmospheric Chemistry and Physics
Refereed publication:Yes
Open Access:Yes
Gold Open Access:Yes
In SCOPUS:Yes
In ISI Web of Science:Yes
DOI :10.5194/acp-14-1055-2014
Page Range:pp. 1055-1073
Publisher:Copernicus Publications
ISSN:1680-7316
Status:Published
Keywords:Arctic stratosphere, nitric acid trihydrate, ozone hole
HGF - Research field:Aeronautics, Space and Transport
HGF - Program:Space
HGF - Program Themes:Earth Observation
DLR - Research area:Raumfahrt
DLR - Program:R EO - Erdbeobachtung
DLR - Research theme (Project):R - Vorhaben Atmosphären- und Klimaforschung
Location: Oberpfaffenhofen
Institutes and Institutions:Institute of Atmospheric Physics > Atmospheric Trace Species
Deposited By: Schlager, Dr.rer.nat. Hans
Deposited On:08 Dec 2014 08:20
Last Modified:02 May 2019 14:04

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