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The global impact of the transport sectors on atmospheric aerosol: simulations for year 2000 emissions

Righi, Mattia and Hendricks, Johannes and Sausen, Robert (2013) The global impact of the transport sectors on atmospheric aerosol: simulations for year 2000 emissions. Atmospheric Chemistry and Physics, 13 (19), pp. 9939-9970. Copernicus Publications. DOI: 10.5194/acp-13-9939-2013 ISSN 1680-7316

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Official URL: http://www.atmos-chem-phys.net/13/9939/2013/acp-13-9939-2013.html

Abstract

We use the EMAC (ECHAM/MESSy Atmospheric Chemistry) global model with the aerosol module MADE (Modal Aerosol Dynamics model for Europe, adapted for global applications) to quantify the impact of transport emissions (land transport, shipping and aviation) on the global aerosol. We consider a present-day (2000) scenario according to the CMIP5 (Climate Model Intercomparison Project Phase 5) emission data set developed in support of the IPCC (Intergovernmental Panel on Climate Change) Fifth Assessment Report. The model takes into account particle mass and number emissions: The latter are derived from mass emissions under different assumptions on the size distribution of particles emitted by the three transport sectors. Additional sensitivity experiments are performed to quantify the effects of the uncertainties behind such assumptions. The model simulations show that the impact of the transport sectors closely matches the emission patterns. Land transport is the most important source of black carbon (BC) pollution in the USA, Europe and the Arabian Peninsula, contributing up to 60–70% of the total surface-level BC concentration in these regions. Shipping contributes about 40–60% of the total aerosol sulfate surface-level concentration along the most-traveled routes of the northern Atlantic and northern Pacific oceans, with a significant impact (~ 10–20%) along the coastlines. Aviation mostly affects aerosol number, contributing about 30–40% of the particle number concentration in the northern midlatitudes' upper troposphere (7–12 km), although significant effects are also simulated at the ground, due to the emissions from landing and take-off cycles. The transport-induced perturbations to the particle number concentrations are very sensitive to the assumptions on the size distribution of emitted particles, with the largest uncertainties (about one order of magnitude) obtained for the land transport sector. The simulated climate impacts, due to aerosol direct and indirect effects, are strongest for the shipping sector, in the range of −222.0 to −153.3 mW m−2, as a consequence of the large impact of sulfate aerosol on low marine clouds and their optical properties.

Item URL in elib:https://elib.dlr.de/84578/
Document Type:Article
Title:The global impact of the transport sectors on atmospheric aerosol: simulations for year 2000 emissions
Authors:
AuthorsInstitution or Email of AuthorsAuthors ORCID iD
Righi, MattiaMattia.Righi (at) dlr.deUNSPECIFIED
Hendricks, JohannesJohannes.Hendricks (at) dlr.deUNSPECIFIED
Sausen, Robertrobert.sausen (at) dlr.deUNSPECIFIED
Date:9 October 2013
Journal or Publication Title:Atmospheric Chemistry and Physics
Refereed publication:Yes
Open Access:Yes
Gold Open Access:Yes
In SCOPUS:Yes
In ISI Web of Science:Yes
Volume:13
DOI :10.5194/acp-13-9939-2013
Page Range:pp. 9939-9970
Publisher:Copernicus Publications
ISSN:1680-7316
Status:Published
Keywords:Aerosol Global modelling Transport impacts
HGF - Research field:Aeronautics, Space and Transport
HGF - Program:Transport
HGF - Program Themes:Transport System
DLR - Research area:Transport
DLR - Program:V VS - Verkehrssystem
DLR - Research theme (Project):V - Verkehrsentwicklung und Umwelt (old)
Location: Oberpfaffenhofen
Institutes and Institutions:Institute of Atmospheric Physics > Atmospheric Dynamics
Deposited By: Righi, Dr. Mattia
Deposited On:04 Nov 2013 09:33
Last Modified:02 May 2019 14:04

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