Application of OMI, SCIAMACHY and GOME-2 satellite SO2 retrievals for detection of large emission sources

Abstract

Retrievals of sulfur dioxide (SO2) from space-based spectrometers are in a relatively early stage of development. Factors such as interference between ozone and SO2 in the retrieval algorithms often lead to errors in the retrieved values. Measurements from the Ozone Monitoring Instrument (OMI), SCanning Imaging Absorption spectroMeter for Atmospheric CHartographY (SCIAMACHY), and Global Ozone Monitoring Experiment -2 (GOME-2) satellite sensors, aver-aged over a period of several years, were used to identify locations with elevated SO2 values and estimate their emission levels. About 30 such locations, detectable by all three sensors and linked to volcanic and anthropogenic sources, were found, after applying low- and high- spatial fre-quency filtration designed to reduce noise and bias and to enhance weak signals to SO2 data from each instrument. Quantitatively, the mean amount of SO2 in the vicinity of the sources, estimated from the three instruments is in general agreement. However a better spatial resolution of OMI makes it possible for this instrument to detect smaller sources and with more details compared to the other two instruments. Over some regions of China, SCIAMACHY and GOME-2 data show mean SO2 values that are almost 1.5 times higher than those from OMI but the suggested spatial filtration technique largely reconciles these differences.