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A fast stratospheric chemistry solver: the E4CHEM submodel for the atmospheric chemistry global circulation model EMAC

Baumgaertner, Andreas J. G. and Jöckel, Patrick and Steil, Benedikt and Tost, Holger and Sander, Rolf (2010) A fast stratospheric chemistry solver: the E4CHEM submodel for the atmospheric chemistry global circulation model EMAC. Geoscientific Model Development, 3, pp. 321-328. Copernicus Publications. DOI: 10.5194/gmd-3-321-2010

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Official URL: http://www.geosci-model-dev.net/3/321/2010/

Abstract

The atmospheric chemistry general circulation model ECHAM5/MESSy (EMAC) and the atmospheric chemistry box model CAABA are extended by a computationally very efficient submodel for atmospheric chemistry, E4CHEM. It focuses on stratospheric chemistry but also includes background tropospheric chemistry. It is based on the chemistry of MAECHAM4-CHEM and is intended to serve as a simple and fast alternative to the flexible but also computationally more demanding submodel MECCA. In a model setup with E4CHEM, EMAC is now also suitable for simulations of longer time scales. The reaction mechanism contains basic O3, CH4, CO, HOx, NOx, and ClOx gas phase chemistry. In addition, E4CHEM includes optional fast routines for heterogeneous reactions on sulphate aerosols and polar stratospheric clouds (substituting the existing submodels PSC and HETCHEM), and scavenging (substituting the existing submodel SCAV). We describe the implementation of E4CHEM into the MESSy structure of CAABA and EMAC. For some species the steady state in the box model differs by up to 100% when compared to results from CAABA/MECCA due to different reaction rates. After an update of the reaction rates in E4CHEM the mixing ratios in both boxmodel and 3-D model simulations are in satisfactory agreement with the results from a simulation where MECCA with a similar chemistry scheme was employed. Finally, a comparison against a simulation with a more complex and already evaluated chemical mechanism is presented in order to discuss shortcomings associated with the simplification of the chemical mechanism.

Item URL in elib:https://elib.dlr.de/66177/
Document Type:Article
Title:A fast stratospheric chemistry solver: the E4CHEM submodel for the atmospheric chemistry global circulation model EMAC
Authors:
AuthorsInstitution or Email of AuthorsAuthors ORCID iD
Baumgaertner, Andreas J. G.MPI for ChemistryUNSPECIFIED
Jöckel, PatrickPatrick.Joeckel (at) dlr.deUNSPECIFIED
Steil, BenediktMPI for ChemistryUNSPECIFIED
Tost, HolgerMPI for ChemistryUNSPECIFIED
Sander, RolfMPI for ChemistryUNSPECIFIED
Date:June 2010
Journal or Publication Title:Geoscientific Model Development
Refereed publication:Yes
Open Access:Yes
Gold Open Access:Yes
In SCOPUS:Yes
In ISI Web of Science:Yes
Volume:3
DOI :10.5194/gmd-3-321-2010
Page Range:pp. 321-328
Publisher:Copernicus Publications
Status:Published
Keywords:Atmospheric Chemistry, Atmospheric Modelling, Stratosphere, Kinetics
HGF - Research field:Aeronautics, Space and Transport (old)
HGF - Program:Space (old)
HGF - Program Themes:W EO - Erdbeobachtung
DLR - Research area:Space
DLR - Program:W EO - Erdbeobachtung
DLR - Research theme (Project):W - Vorhaben Atmosphären- und Klimaforschung (old)
Location: Oberpfaffenhofen
Institutes and Institutions:Institute of Atmospheric Physics > Atmospheric Dynamics
Deposited By: Jöckel, Dr. Patrick
Deposited On:15 Nov 2010 18:16
Last Modified:02 May 2019 14:13

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