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Idealized Glass Transitions under Pressure: Dynamics versus Thermodynamics

Voigtmann, Thomas (2008) Idealized Glass Transitions under Pressure: Dynamics versus Thermodynamics. Physical Review Letters, 101, 095701. doi: 10.1103/PhysRevLett.101.095701.

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Official URL: http://link.aps.org/abstract/PRL/v101/e095701

Abstract

The interplay of slow dynamics and thermodynamic features of dense liquids is studied by examining how the glass transition changes depending on the presence or absence of Lennard-Jones-like attractions. Quite different thermodynamic behavior leaves the dynamics unchanged, with important consequences for high-pressure experiments on glassy liquids. Numerical results are obtained within mode-coupling theory (MCT), but the qualitative features are argued to hold more generally. A simple square-well model can be used to explain generic features found in experiment.

Item URL in elib:https://elib.dlr.de/55572/
Document Type:Article
Title:Idealized Glass Transitions under Pressure: Dynamics versus Thermodynamics
Authors:
AuthorsInstitution or Email of AuthorsAuthor's ORCID iDORCID Put Code
Voigtmann, ThomasUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Date:28 August 2008
Journal or Publication Title:Physical Review Letters
Refereed publication:Yes
Open Access:No
Gold Open Access:No
In SCOPUS:No
In ISI Web of Science:Yes
Volume:101
DOI:10.1103/PhysRevLett.101.095701
Page Range:095701
Status:Published
Keywords:glass transition, mode coupling theory, high-pressure experiments
HGF - Research field:Aeronautics, Space and Transport (old)
HGF - Program:Space (old)
HGF - Program Themes:W FR - Forschung unter Weltraumbedingungen (old)
DLR - Research area:Space
DLR - Program:W FR - Forschung unter Weltraumbedingungen
DLR - Research theme (Project):W - Vorhaben Materialwissenschaftliche Forschung (old)
Location: Köln-Porz
Institutes and Institutions:Institute of Materials Physics in Space
Deposited By: Voigtmann, Dr.rer.nat. Thomas
Deposited On:20 Oct 2008
Last Modified:27 Apr 2009 15:16

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