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Preparation and characterization of carbon aerogels as electrode materials for battery applications

Dzierbinski, Adam and Kröner, Jessica and Schwan, Marina and Kaiser, Christian and Merz, Holger and Milow, Barbara (2023) Preparation and characterization of carbon aerogels as electrode materials for battery applications. 2nd International Congress on Aerogel Inspired Materials, 2023-09-26 - 2023-09-29, Donostia – San Sebastían, Spain.

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Abstract

The production of lithium ion batteries is very resource-intensive and undergoes continuous growth in the face of increasing electrification in the energy and mobility sector as well as other areas that contribute to our current living standard. Next to lithium, graphite is one of the main materials required for battery production and is currently mined on a big scale from natural deposits causing the emission of toxic nanoscopic particles. On the other hand, preparation of synthetic graphite causes high carbon emissions as it requires a high energy-input.[1] In order to replace graphite and reduce current production effects on the environment, this work deals with the preparation and characterization of novel composite materials applicable in anodes. These composites consist of carbonized chitosan aerogels and carbon black that has been recovered and highly purified in a sophisticated process from end-of-life tyres, thus contributing to an overall more sustainable rechargeable battery. In this work, carbon aerogels have been obtained via carbonization of previously prepared chitosan aerogels[2]. The influence of various preparation conditions (applied temperature, atmosphere) on the pore structure (scanning electron microscopy, surface area, pore volume, pore size distribution), elemental composition and electrical conductivity has been studied and compared. Various approaches for material activation such as the application of CO2 have been tested. Furthermore, the influence of post-synthetic processing steps (milling, application of pressure) performed during electrode production has been investigated on the quest towards an optimised anode material. [1] Gomez-Martin, A.; Martinez-Fernandez, J.; Ruttert, M.; Heckmann, A.; Winter, M.; Placke, T.; Ramirez-Rico, J., Iron-Catalyzed Graphitic Carbon Materials from Biomass Resources as Anodes for Lithium-Ion Batteries. ChemSusChem 2018, 11 (16), 2776-2787. [2] Preibisch, I.; Niemeyer, P.; Yusufoglu, Y.; Gurikov, P.; Milow, B.; Smirnova, I. Polysaccharide-Based Aerogel Bead Production via Jet Cutting Method. Materials 2018, 11, 1287.

Item URL in elib:https://elib.dlr.de/198030/
Document Type:Conference or Workshop Item (Speech)
Title:Preparation and characterization of carbon aerogels as electrode materials for battery applications
Authors:
AuthorsInstitution or Email of AuthorsAuthor's ORCID iDORCID Put Code
Dzierbinski, AdamUNSPECIFIEDhttps://orcid.org/0000-0002-9004-2989UNSPECIFIED
Kröner, JessicaUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Schwan, MarinaUNSPECIFIEDhttps://orcid.org/0000-0001-6329-8164UNSPECIFIED
Kaiser, ChristianUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Merz, HolgerUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Milow, BarbaraUNSPECIFIEDhttps://orcid.org/0000-0002-6350-7728UNSPECIFIED
Date:September 2023
Refereed publication:Yes
Open Access:No
Gold Open Access:No
In SCOPUS:No
In ISI Web of Science:No
Status:Published
Keywords:carbon aerogels, chitosan aerogel, electrical conductivity, electrode material, Li-ion battery
Event Title:2nd International Congress on Aerogel Inspired Materials
Event Location:Donostia – San Sebastían, Spain
Event Type:international Conference
Event Start Date:26 September 2023
Event End Date:29 September 2023
HGF - Research field:Energy
HGF - Program:Materials and Technologies for the Energy Transition
HGF - Program Themes:Electrochemical Energy Storage
DLR - Research area:Energy
DLR - Program:E VS - Combustion Systems
DLR - Research theme (Project):E - Materials for Electrochemical Energy Storage
Location: Köln-Porz
Institutes and Institutions:Institute of Materials Research > Aerogels and Aerogel Composites
Deposited By: Schwan, Marina
Deposited On:06 Nov 2023 10:18
Last Modified:24 Apr 2024 20:58

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