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Beneficial Effects of Three-Dimensional Structured Electrodes for the Fast Charging of Lithium-Ion Batteries

De Lauri, Vittorio and Krumbein, Lukas and Hein, Simon and Prifling, Benedikt and Schmidt, Volker and Danner, Timo and Latz, Arnulf (2021) Beneficial Effects of Three-Dimensional Structured Electrodes for the Fast Charging of Lithium-Ion Batteries. ACS Applied Energy Materials. American Chemical Society (ACS). doi: 10.1021/acsaem.1c02621. ISSN 2574-0962. (In Press)

[img] PDF - Only accessible within DLR bis 1 January 2023 - Preprint version (submitted draft)

Official URL: https://pubs.acs.org/doi/abs/10.1021/acsaem.1c02621


Lithium-ion batteries are the dominating electrochemical energy storage technology for battery electric vehicles. However, additional optimization is needed to meet the requirements of the automotive industry regarding energy density, cost, safety, and fast charging performance. In conventional electrode designs, there is a trade-off between energy density and rate capability. Recently, three-dimensional (3D) structuring techniques, such as laser perforation, were proposed to optimize both properties at the same time and remarkable improvements in fast-charging performance have been demonstrated. In this work, we investigate the effect of structuring techniques on the thermal properties and electrochemical performance of the battery using microstructure-resolved simulations. Particular attention will be paid to the heat evolution and lithium plating during fast charging of the batteries. According to our results, 3D structuring is able to reduce the overall cell resistance by improving the electrolyte transport. This has a positive impact on the fast charging capability of the cell and, moreover, reduces the danger of lithium plating.

Item URL in elib:https://elib.dlr.de/147597/
Document Type:Article
Title:Beneficial Effects of Three-Dimensional Structured Electrodes for the Fast Charging of Lithium-Ion Batteries
AuthorsInstitution or Email of AuthorsAuthor's ORCID iD
De Lauri, VittorioUniversità degli studi di Modena e Reggio EmiliaUNSPECIFIED
Krumbein, Lukaslukas.krumbein (at) dlr.deUNSPECIFIED
Hein, SimonSimon.Hein (at) dlr.dehttps://orcid.org/0000-0002-6728-9983
Prifling, BenediktUniversity of Ulmhttps://orcid.org/0000-0002-2952-0208
Schmidt, VolkerUniversity of UlmUNSPECIFIED
Danner, TimoTimo.Danner (at) dlr.dehttps://orcid.org/0000-0003-2336-6059
Latz, ArnulfArnulf.Latz (at) dlr.deUNSPECIFIED
Date:8 December 2021
Journal or Publication Title:ACS Applied Energy Materials
Refereed publication:Yes
Open Access:No
Gold Open Access:No
In ISI Web of Science:Yes
DOI :10.1021/acsaem.1c02621
Publisher:American Chemical Society (ACS)
Status:In Press
Keywords:lithium-ion battery microstructure-resolved simulation fast charging laser perforation lithium plating
HGF - Research field:Aeronautics, Space and Transport
HGF - Program:Transport
HGF - Program Themes:Transport System
DLR - Research area:Transport
DLR - Program:V VS - Verkehrssystem
DLR - Research theme (Project):V - Energie und Verkehr
Location: Ulm
Institutes and Institutions:Institute of Engineering Thermodynamics > Computational Electrochemistry
Deposited By: Danner, Timo
Deposited On:23 Dec 2021 21:13
Last Modified:23 Dec 2021 21:13

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