Rizzo, T. und Voigtmann, Th. (2015) Qualitative features at the glass crossover. Europhysics Letters, 111, Seite 56008. EPLA. doi: 10.1209/0295-5075/111/56008. ISSN 0295-5075.
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Kurzfassung
We discuss generic features of the dynamics of glass-forming liquids close to the glass transition singularity of the idealized mode-coupling theory (MCT). The analysis is based on a recent theory by one of the authors for the intermediate-time dynamics ($\beta$ relaxation), derived by applying dynamical field-theory techniques to the idealized MCT. Taking the long-time asymptote of the $\beta$-relaxation regime as a proxy for universal aspects of the slow structural ($\alpha$) relaxation, we explain three prominent features of the dynamical crossover: the change from a power-law to exponential increase in the structural relaxation time, the replacement of the Stokes-Einstein relation between diffusion and viscosity by a fractional law, and two distinct growth regimes of the thermal susceptibility that has been associated to dynamical heterogeneities.
elib-URL des Eintrags: | https://elib.dlr.de/99742/ | ||||||||||||
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Dokumentart: | Zeitschriftenbeitrag | ||||||||||||
Titel: | Qualitative features at the glass crossover | ||||||||||||
Autoren: |
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Datum: | 2015 | ||||||||||||
Erschienen in: | Europhysics Letters | ||||||||||||
Referierte Publikation: | Ja | ||||||||||||
Open Access: | Nein | ||||||||||||
Gold Open Access: | Nein | ||||||||||||
In SCOPUS: | Ja | ||||||||||||
In ISI Web of Science: | Ja | ||||||||||||
Band: | 111 | ||||||||||||
DOI: | 10.1209/0295-5075/111/56008 | ||||||||||||
Seitenbereich: | Seite 56008 | ||||||||||||
Verlag: | EPLA | ||||||||||||
ISSN: | 0295-5075 | ||||||||||||
Status: | veröffentlicht | ||||||||||||
Stichwörter: | mode coupling theory, glass transition, replica theory | ||||||||||||
HGF - Forschungsbereich: | Luftfahrt, Raumfahrt und Verkehr | ||||||||||||
HGF - Programm: | Raumfahrt | ||||||||||||
HGF - Programmthema: | Forschung unter Weltraumbedingungen | ||||||||||||
DLR - Schwerpunkt: | Raumfahrt | ||||||||||||
DLR - Forschungsgebiet: | R FR - Forschung unter Weltraumbedingungen | ||||||||||||
DLR - Teilgebiet (Projekt, Vorhaben): | R - Vorhaben Materialwissenschaftliche Forschung (alt) | ||||||||||||
Standort: | Köln-Porz | ||||||||||||
Institute & Einrichtungen: | Institut für Materialphysik im Weltraum | ||||||||||||
Hinterlegt von: | Voigtmann, Dr.rer.nat. Thomas | ||||||||||||
Hinterlegt am: | 24 Nov 2015 09:24 | ||||||||||||
Letzte Änderung: | 10 Jan 2019 15:47 |
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