Rizzo, T. und Voigtmann, Th. (2015) Qualitative features at the glass crossover. Europhysics Letters, 111, Seite 56008. EPLA. doi: 10.1209/0295-5075/111/56008. ISSN 0295-5075.
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Kurzfassung
We discuss generic features of the dynamics of glass-forming liquids close to the glass transition singularity of the idealized mode-coupling theory (MCT). The analysis is based on a recent theory by one of the authors for the intermediate-time dynamics ($\beta$ relaxation), derived by applying dynamical field-theory techniques to the idealized MCT. Taking the long-time asymptote of the $\beta$-relaxation regime as a proxy for universal aspects of the slow structural ($\alpha$) relaxation, we explain three prominent features of the dynamical crossover: the change from a power-law to exponential increase in the structural relaxation time, the replacement of the Stokes-Einstein relation between diffusion and viscosity by a fractional law, and two distinct growth regimes of the thermal susceptibility that has been associated to dynamical heterogeneities.
| elib-URL des Eintrags: | https://elib.dlr.de/99742/ | ||||||||||||
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| Dokumentart: | Zeitschriftenbeitrag | ||||||||||||
| Titel: | Qualitative features at the glass crossover | ||||||||||||
| Autoren: |
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| Datum: | 2015 | ||||||||||||
| Erschienen in: | Europhysics Letters | ||||||||||||
| Referierte Publikation: | Ja | ||||||||||||
| Open Access: | Nein | ||||||||||||
| Gold Open Access: | Nein | ||||||||||||
| In SCOPUS: | Ja | ||||||||||||
| In ISI Web of Science: | Ja | ||||||||||||
| Band: | 111 | ||||||||||||
| DOI: | 10.1209/0295-5075/111/56008 | ||||||||||||
| Seitenbereich: | Seite 56008 | ||||||||||||
| Verlag: | EPLA | ||||||||||||
| ISSN: | 0295-5075 | ||||||||||||
| Status: | veröffentlicht | ||||||||||||
| Stichwörter: | mode coupling theory, glass transition, replica theory | ||||||||||||
| HGF - Forschungsbereich: | Luftfahrt, Raumfahrt und Verkehr | ||||||||||||
| HGF - Programm: | Raumfahrt | ||||||||||||
| HGF - Programmthema: | Forschung unter Weltraumbedingungen | ||||||||||||
| DLR - Schwerpunkt: | Raumfahrt | ||||||||||||
| DLR - Forschungsgebiet: | R FR - Forschung unter Weltraumbedingungen | ||||||||||||
| DLR - Teilgebiet (Projekt, Vorhaben): | R - Vorhaben Materialwissenschaftliche Forschung (alt) | ||||||||||||
| Standort: | Köln-Porz | ||||||||||||
| Institute & Einrichtungen: | Institut für Materialphysik im Weltraum | ||||||||||||
| Hinterlegt von: | Voigtmann, Dr.rer.nat. Thomas | ||||||||||||
| Hinterlegt am: | 24 Nov 2015 09:24 | ||||||||||||
| Letzte Änderung: | 10 Jan 2019 15:47 |
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