Harrer, Ch. J. und Puertas, A. M. und Voigtmann, Th. und Fuchs, M. (2012) Probability Densities of a Forced Probe Particle in Glass: Results from Mode Coupling Theory and Simulations of Active Microrheology. Zeitschrift für Physikalische Chemie, 226, Seiten 779-795. de Gruyter. doi: 10.1524/zpch.2012.0275.
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Kurzfassung
We investigate the displacements of a probe particle inside a glass, when a strong external force is applied to the probe (active nonlinear microrheology). Calculations within mode coupling theory are presented for glasses of hard spheres and compared to Langevin and Brownian dynamics simulations. Under not too strong forces where the probe remains trapped, the probe density distribution becomes anisotropic. It is shifted towards the direction of the force, develops an enhanced tail in that direction (signaled by a positive skewness), and exhibits different variances along and perpendicular to the force direction. A simple model of an harmonically trapped probe rationalizes the low force limit, with strong strain softening setting in at forces of the order of a few thermal energies per particle radius.
elib-URL des Eintrags: | https://elib.dlr.de/77548/ | ||||||||||||||||||||
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Dokumentart: | Zeitschriftenbeitrag | ||||||||||||||||||||
Titel: | Probability Densities of a Forced Probe Particle in Glass: Results from Mode Coupling Theory and Simulations of Active Microrheology | ||||||||||||||||||||
Autoren: |
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Datum: | September 2012 | ||||||||||||||||||||
Erschienen in: | Zeitschrift für Physikalische Chemie | ||||||||||||||||||||
Open Access: | Nein | ||||||||||||||||||||
Gold Open Access: | Nein | ||||||||||||||||||||
In SCOPUS: | Ja | ||||||||||||||||||||
In ISI Web of Science: | Ja | ||||||||||||||||||||
Band: | 226 | ||||||||||||||||||||
DOI: | 10.1524/zpch.2012.0275 | ||||||||||||||||||||
Seitenbereich: | Seiten 779-795 | ||||||||||||||||||||
Verlag: | de Gruyter | ||||||||||||||||||||
Status: | veröffentlicht | ||||||||||||||||||||
Stichwörter: | micro-rheology, mode coupling theory, local elastic constants | ||||||||||||||||||||
HGF - Forschungsbereich: | Verkehr und Weltraum (alt) | ||||||||||||||||||||
HGF - Programm: | Weltraum (alt) | ||||||||||||||||||||
HGF - Programmthema: | W FR - Forschung unter Weltraumbedingungen (alt) | ||||||||||||||||||||
DLR - Schwerpunkt: | Weltraum | ||||||||||||||||||||
DLR - Forschungsgebiet: | W FR - Forschung unter Weltraumbedingungen | ||||||||||||||||||||
DLR - Teilgebiet (Projekt, Vorhaben): | W - Vorhaben Materialwissenschaftliche Forschung (alt) | ||||||||||||||||||||
Standort: | Köln-Porz | ||||||||||||||||||||
Institute & Einrichtungen: | Institut für Materialphysik im Weltraum | ||||||||||||||||||||
Hinterlegt von: | Voigtmann, Dr.rer.nat. Thomas | ||||||||||||||||||||
Hinterlegt am: | 02 Okt 2012 08:40 | ||||||||||||||||||||
Letzte Änderung: | 06 Sep 2019 15:30 |
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